GUI Tool for PostgreSQL

There is a comprehensive list of tools on the PostgreSQL Wiki:

https://wiki.postgresql.org/wiki/PostgreSQL_Clients

And of course PostgreSQL itself comes with pgAdmin, a GUI tool for accessing Postgres databases.

Postgres Enterprise Manager from EnterpriseDB is probably the most advanced you'll find. It includes all the features of pgAdmin, plus monitoring of your hosts and database servers, predictive reporting, alerting and a SQL Profiler.

http://www.enterprisedb.com/products-services-training/products/postgres-enterprise-manager

Ninja edit disclaimer/notice: it seems that this user is affiliated with EnterpriseDB, as the linked Postgres Enterprise Manager website contains a video of one Dave Page.