Creating JSON on the fly with JObject

Well, how about:

dynamic jsonObject = new JObject();
jsonObject.Date = DateTime.Now;
jsonObject.Album = "Me Against the world";
jsonObject.Year = 1995;
jsonObject.Artist = "2Pac";

Neither dynamic, nor JObject.FromObject solution works when you have JSON properties that are not valid C# variable names e.g. "@odata.etag". I prefer the indexer initializer syntax in my test cases:

JObject jsonObject = new JObject
{
    ["Date"] = DateTime.Now,
    ["Album"] = "Me Against The World",
    ["Year"] = 1995,
    ["Artist"] = "2Pac"
};

Having separate set of enclosing symbols for initializing JObject and for adding properties to it makes the index initializers more readable than classic object initializers, especially in case of compound JSON objects as below:

JObject jsonObject = new JObject
{
    ["Date"] = DateTime.Now,
    ["Album"] = "Me Against The World",
    ["Year"] = 1995,
    ["Artist"] = new JObject
    {
        ["Name"] = "2Pac",
        ["Age"] = 28
    }
};

With object initializer syntax, the above initialization would be:

JObject jsonObject = new JObject
{
    { "Date", DateTime.Now },
    { "Album", "Me Against The World" },
    { "Year", 1995 }, 
    { "Artist", new JObject
        {
            { "Name", "2Pac" },
            { "Age", 28 }
        }
    }
};

You can use the JObject.Parse operation and simply supply single quote delimited JSON text.

JObject  o = JObject.Parse(@"{
  'CPU': 'Intel',
  'Drives': [
    'DVD read/writer',
    '500 gigabyte hard drive'
  ]
}");

This has the nice benefit of actually being JSON and so it reads as JSON.

Or you have test data that is dynamic you can use JObject.FromObject operation and supply a inline object.

JObject o = JObject.FromObject(new
{
    channel = new
    {
        title = "James Newton-King",
        link = "http://james.newtonking.com",
        description = "James Newton-King's blog.",
        item =
            from p in posts
            orderby p.Title
            select new
            {
                title = p.Title,
                description = p.Description,
                link = p.Link,
                category = p.Categories
            }
    }
});

Json.net documentation for serialization

There are some environment where you cannot use dynamic (e.g. Xamarin.iOS) or cases in where you just look for an alternative to the previous valid answers.

In these cases you can do:

using Newtonsoft.Json.Linq;

JObject jsonObject =
     new JObject(
             new JProperty("Date", DateTime.Now),
             new JProperty("Album", "Me Against The World"),
             new JProperty("Year", "James 2Pac-King's blog."),
             new JProperty("Artist", "2Pac")
         )

More documentation here: http://www.newtonsoft.com/json/help/html/CreatingLINQtoJSON.htm